Hmm, I had basically the same question with a different use case.
I stepped up a few prints with a 1.0 mm nozzle, which is great for printing walls at 0.8 layer height, but the top/bottom get a bit thick. It would be nice to be able to thing them out a bit by using smaller layers.
Cura currently has an option to have the initial layer a different height then the rest, so it doesn't seem to far off to have an option to setting the top/bottom to a different layer.
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ahoeben 1,591
The simple answer - unsatisfying as it may be - is that Cura does not have functionality to let you do that easily. You would have to mix gcode files manually.
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